Please wait a minute...
浙江大学学报(工学版)
环境工程     
等离子体联合光催化治理喷漆废气
邵振华, 魏博伦, 叶志平, 何奕, 施耀
浙江大学 化学工程与生物工程学系,生物质化工教育部重点实验室,浙江 杭州 310028
Treatment of exhaust gas from spray paint process with plasma-photocatalytic method
SHAO Zhen-hua, WEI Bo-lun, YE Zhi-ping, HE Yi, SHI Yao
Department of Chemical and Biological Engineering,Key Laboratory of Biomass Chemical Engineering of Ministry of Education, Zhejiang University, Hangzhou 310028, China
 全文: PDF(1041 KB)  
摘要:

针对木门制造业喷涂过程产生的有机废气,探究利用等离子体联合催化降解有机废气的机理与工程应用可行性,并探索涂装废气降解装置的最优组合方式.在实验室小试和工业中试的基础上,研发一套处理5 000 m3/h的涂装废气等离子体联合光催化装置.该废气处理装置可使总可挥发性有机物和二甲苯的降解率分别达到70%和60%以上,治理示范工程的调试和运行结果表明该技术的运行成本较低.通过对木业涂装排放的有机废气进行低能耗、高去除率的无害化处理后,实现了废气的达标排放.因此,该装置可作为一种解决涂装过程中有机废气污染问题新的手段.

关键词: 等离子体喷漆废气二甲苯有机废气光催化    
Abstract:

Plasma-photocatalytic technique was applied to decompose the volatile organic compounds (VOCs) from the painting process of the wooden doors manufacturing. The synergetic effect of the plasma-catalysis and its industrial feasibility were investigated, moreover, the operating conditions and the combination of exhaust gas treating process were optimized. A plasma-catalytic configuration capable of dealing with VOCs exhaust at a rate of 5 000 m3/h was developed on the basis of laboratory test and industrial pilot. The degradation ratio of total VOCs and xylene can go beyond 70% and 60%, respectively. The results also showed that the operating cost of the process is in a relatively low range. Thus, with this method, a high degradation rate that meets the national emission standards can be achieved at a relatively low cost. This process provides a new highly effective alternative to the conventional methods for the removal of VOCs from the painting process of the wooden doors manufacturing.

Key words: photo-catalysis    VOCs    paint exhaust    plasma    xylene
出版日期: 2014-07-04
:  X 788  
基金资助:

林业公益性行业科研专项经费资助项目(201204703);浙江省自然科学基金重点资助项目(LZ12E08002).

通讯作者: 施耀,男,教授.     E-mail: shiyao@zju.edu.cn
作者简介: 邵振华(1979—),男,高级工程师.E-mail: zhenhua_shao@163.com
服务  
把本文推荐给朋友
加入引用管理器
E-mail Alert
RSS
作者相关文章  
施耀
魏博伦
邵振华
叶志平
何奕

引用本文:

邵振华, 魏博伦, 叶志平, 何奕, 施耀. 等离子体联合光催化治理喷漆废气[J]. 浙江大学学报(工学版), 10.3785/j.issn.1008-973X.2014.06.023.

SHAO Zhen-hua, WEI Bo-lun, YE Zhi-ping, HE Yi, SHI Yao. Treatment of exhaust gas from spray paint process with plasma-photocatalytic method. JOURNAL OF ZHEJIANG UNIVERSITY (ENGINEERING SCIENCE), 10.3785/j.issn.1008-973X.2014.06.023.

链接本文:

http://www.zjujournals.com/xueshu/eng/CN/10.3785/j.issn.1008-973X.2014.06.023        http://www.zjujournals.com/xueshu/eng/CN/Y2014/V48/I6/1127

[1] 郝明途,林天佳,刘焱,等.我国PM2.5的污染状况和污染特征[J].环境科学与管理,2006,31(2): 58-61.
HAO Tu-ming, LIN Tian-jia, LIU Yan, et al. PM2.5 pollution condition and characteristics of our country[J]. Environmental Science and Management,2006,31(2): 58-61.
[2] 吴文锋.VOCs处理技术研究与展望[J].城市建设,2010,10: 100-101.
WU Wen-feng. VOCs processing technology research and prospects[J].China City Construction,2010,10: 100-101.
[3] 郭建光,李忠,奚红霞,等.超声浸渍法对CuO/CeO2/γ-Al2O3催化剂催化燃烧挥发性有机化合物性能的影响[J].化工学报,2006,57(4): 815-820.
GUO Jian-guang, LI Zhong, XI Hong-xia, et al. Effect of Preparation by ultrasound-assisted impregnation on Properties of CuO/CeO2/γ-Al2O3 catalysts for catalytic combustion of VOCs[J].Journal of Chemical Industry and Engineering (China). 2006,57(4): 815-820.
[4] 宁晓宇,陈红,耿静,等.低温等离子体-催化协同空气净化技术研究进展[J].科技导报,2009,27(6): 97-101.
NING Xiao-yu, CHEN Hong, GENG Jing, et al.Advances in researches on catalysis-assisted non-thermalplasma technology for air pollution control[J]. Science & Technology Review,2009,27(6): 97-101.
[5] 邱作志,叶代启.放电等离子体驱动光催化降解甲苯研究[J].工业催化,2008,16(6): 69-74.
QIU Zuo-zhi, YE Dai-qi. Discharge plasma driven research on photocatalytic degradation of toluene[J].Industrial Catalysis,2008,16(6): 69-74.
[6] JIM V D, JO D, CHRISTOPHE L. Combining non-thermal plasma with heterogeneous catalysis in waste gas treatment: A review[J]. Applied Catalysis B: Environmental, 2008,78: 324-333.
[7] HSIN L, CHEN How, LEE Ming, et al. Removal of volatile organic compounds by single-stage and two-stage plasma catalysis systems: a review of the performance enhancement mechanisms, current status, and suitable applications[J]. Environmental Science & Technology, 2009,43: 2216-2227.
[8] 程萍,顾明元,金燕苹,等.TiO2光催化剂可见光化研究进展[J].化学进展,2005,17(1): 8-14.
CHENG Ping, GU Ming-yuan, JIN Yan-ping, et al. Recent progress in titania photocatalyst operating in visible light[J]. Progress in Chemistry, 2005,17(1): 8-14.
[9] 阮建军,潘维龙,施耀.非平衡等离子体脱臭技术研究进展[J].化工进展,2006,25(1): 35-38.
RUAN Jian-jun, PAN Wei-long, SHI Yao. Research advances of nonthermal plasma for odor removal[J]. Chemical Industry and Engineering Progress,2006,25(1): 35-38.
[10] CHEN Jie, YANG Jian-tao, SHI Yao, et al. Abatement of malodorants from pesticide factory in dielectric barrier discharges[J]. Journal of Hazardous Materials, 2010,177: 908-913.
[11] YE Zhi-ping, WANG Chun-xia, SHI Yao, et al. A novel dielectric barrier discharge reactor with photocatalytic electrode based on sintered metal fibers for abatement of xylene[J]. Journal of Hazardous Materials, 2012,241242: 216-223.
[12] 李爽,沈隽,江淑敏,等.不同外部环境因素下胶合板VOCs的释放特性[J].林业科学,2013,49(1): 179-184.
LI Shuang, SHEN Jun, JIANG Shu-min, et al. Characteristics of VOC Emission from Plywood in Different Environment Factors[J].Scientia Silvae Sinicae, 2013,49(1): 179-184.
[13] THEVENET F, GUAITELLA O, et al. Influence of water vapour on plasma photocatalytic oxidation efficiency of acetylene[J]. Applied Catalysis B: Environmental, 2008,84: 813-820.

[1] 刘楠, 滕富华, 陆建海, 董事壁, 顾震宇. 光催化-吸收法处理家具涂装废气中试试验[J]. 浙江大学学报(工学版), 2017, 51(2): 393-398.
[2] 尚建丽, 宗志芳. 基于湿效应Ce-La/TiO2空心微球制备及光-湿性能[J]. 浙江大学学报(工学版), 2017, 51(2): 304-311.
[3] 徐辉, 蔡忆昔, 李小华, 施蕴曦, 李伟俊 . 低温等离子体降低柴油机微粒和NOx排放试验研究[J]. 浙江大学学报(工学版), 2016, 50(12): 2418-2423.
[4] 邱坤赞,耿雪威,蔡宇翔,竺新波,郑成航,高翔. 等离子体协同V2O5 WO3/TiO2催化降解恶臭气体的试验研究[J]. 浙江大学学报(工学版), 2016, 50(1): 63-69.
[5] 李秋顺,成荣,张旭霖,陈燕,史建国,李明宇,于永江,董文飞. 聚合物薄膜对表面等离子体共振光谱的调制[J]. 浙江大学学报(工学版), 2015, 49(9): 1796-1804.
[6] 张连成, 黄逸凡, 刘振, 闫克平. 水静压对脉冲放电及深拖等离子体震源的影响[J]. 浙江大学学报(工学版), 2015, 49(7): 1395-1400.
[7] 郑超,徐羽贞,黄逸凡,刘振,闫克平. 脉冲等离子体射流杀灭表面和水中的细菌[J]. 浙江大学学报(工学版), 2014, 48(7): 1329-1335.
[8] 张云卿, 李晓东, 杜长明, 孙晓明, 任咏, 严建华. 磁旋转滑动弧电参数与电弧图像分析[J]. J4, 2013, 47(4): 687-691.
[9] 陈永铎, 王晓晨, 李颖, 朱安娜, 刘振, 闫克平. 等离子体辅助Fenton洗消甲基膦酸二甲酯水溶液[J]. J4, 2013, 47(12): 2195-2201.
[10] 倪明江, 程奎, 余量, 李晓东, 陆胜勇, 严建华. 逆向涡流等离子体降解飞灰中二恶英的研究[J]. J4, 2012, 46(4): 584-589.
[11] 彭盛华, 张欣, 何建军. 氩等离子体诱导量子阱混合技术[J]. J4, 2011, 45(6): 1057-1061.
[12] 王勤, 严建华, 潘新潮, 池涌, 高飞. 利用热等离子体熔融垃圾焚烧飞灰[J]. J4, 2011, 45(1): 141-145.
[13] 杨建涛, 潘华, 陈杰, 苏清发, 汪大翚, 施耀. 低温等离子体吸附两段式系统降解硫化氢[J]. J4, 2010, 44(12): 2411-2415.
[14] 郦雅平, 王晓萍, 赵光灿, 詹舒越, 刘玉玲. SPR光谱信号的一阶矩数据分析方法[J]. J4, 2010, 44(12): 2269-2273.
[15] 严建华, 刘亚纳, 李晓东, 等. 不同气氛下气液两相滑动弧放电降解甲基紫[J]. J4, 2009, 43(5): 931-936.