Please wait a minute...
浙江大学学报(工学版)
环境与能源工程     
化纤行业PM2.5和VOCs排放特性研究
陈文聪, 侯艺文, 吴建, 王莉红
1. 浙江大学 环境与资源学院,浙江 杭州 310058
2. 浙江省环境保护科学设计研究院,浙江 杭州 310007
Characteristics of PM2.5 and VOCs emission from chemical fiber industry
CHEN Wen cong, HOU Yi wen, WU Jian, WANG Li hong
1. College of Environmental and Resource Sciences, Zhejiang University, Hangzhou 310058, China;
2. Environmental Science Research and Design Institute of Zhejiang, Hangzhou 310007, China
 全文: PDF(2043 KB)   HTML
摘要:

以化纤行业为研究对象,采用本地排放因子,按时间、空间、子行业分别建立VOCs的源排放清单,应用Salford Predictive Miner(SPM)数据挖掘工具分析浙江省化纤行业污染物排放特征,分析PM2.5和VOCs以及其他大气污染因子(NOx、SO2、PM10、CO)之间的关联性.结果显示,近年来我国化纤行业VOCs排放量快速上升,子行业中人造纤维VOCs排放量占比超过60%.在浙江省化纤行业中,低浓度的VOCs排放会对PM2.5排放量产生极敏感的影响,对PM2.5排放量影响最大的是NOx的排放量.制定化纤行业大气污染控制措施和政策时,加强控制NOx排放总量和VOCs排放浓度十分必要.

Abstract:

Chemical fiber industry in China was discussed by using local emission factors and its VOCs emission inventories were constructed via time, space and subsectors, respectively. Both emission characteristics and correlations between particle matter with diameter of less than 2.5 μm (PM2.5), VOCs and other factors (NOx, SO2, PM10, CO and regions, sub-sectors) were presented with the Salford Predictive Miner. Results showed that VOCs emission from chemical fiber industry in China had a rapid rise in recent years. Rayon was recognized as the key VOCs emission source for chemical fiber industries, accounting for more than 60% of total VOCs. For Zhejiang province, NOx emission reduction played a key role for controlling PM2.5 index values. A large amount of low concentrations VOCs emissions should be limited for keeping a small PM2.5 index. More attention should be paid on the control of total NOx emissions amount and VOCs emission concentrations when developing air pollution control measures and policies in chemical fiber industry.

出版日期: 2017-01-01
CLC:  X 511  
基金资助:

国家“863”高技术研究发展计划资助项目(SS2013AA0616).

通讯作者: 王莉红,女,副教授. ORCID:0000-0001-7056-7318.     E-mail: wanglh@zju.edu.cn
作者简介: 陈文聪(1993—),女,硕士生,从事环境规划与管理研究. ORCID: 0000-0002-2196-1308. E-mail:chenwencong@zju.edu.cn
服务  
把本文推荐给朋友
加入引用管理器
E-mail Alert
作者相关文章  

引用本文:

陈文聪, 侯艺文, 吴建, 王莉红. 化纤行业PM2.5和VOCs排放特性研究[J]. 浙江大学学报(工学版), 10.3785/j.issn.1008-973X.2017.01.018.

CHEN Wen cong, HOU Yi wen, WU Jian, WANG Li hong. Characteristics of PM2.5 and VOCs emission from chemical fiber industry. JOURNAL OF ZHEJIANG UNIVERSITY (ENGINEERING SCIENCE), 10.3785/j.issn.1008-973X.2017.01.018.

[1] 中华人民共和国国家统计局.2015年国民经济和社会发展统计公报[EB/OL].[2016-02-29]. http:∥www.stats.gov.cn/tjsj/zxfb/201602/ t20160229_1323991.html.
[2] 陈颖,叶代启,刘秀珍,等.我国工业源VOCs排放的源头追踪和行业特征研究[J].中国环境科学,2012,32(01): 48-55.
CHEN Ying, YE Daiqi, LIU Xiuzhen, et al. Source tracing and characteristics of industrial VOCs emissions in China [J]. China Environmental Science, 2012,32(01): 48-55.
[3] 龚芳.我国人为源VOCs排放清单及行业排放特征分析[D].西安:西安建筑科技大学,2013.
GONG Fang. Anthropogenic volatile organic compounds emission inventory and characteristics in China [D].Xi’an: Xi’an University of Architecture and Technology,2013.
[4] 黄薇薇.我国工业源挥发性有机化合物排放特征及其控制技术评估研究[D].杭州:浙江大学, 2016.
HUANG Weiwei. Characteristics of industrial VOCsemissions and evaluation of control technology in China [D]. Hangzhou: Zhejiang University, 2016.
[5] 中国产业信息网.2014年112月全国化学纤维产量分省市统计表[R/OL].[20150401]. http:∥www.chyxx.com/data/201504/309390.html.
[6] 余宇帆,卢清,郑君瑜,等.珠江三角洲地区重点VOC排放行业的排放清单[J].中国环境科学, 2011, 31(02): 195-201.
YU Yufan, LU Qing, ZHENG Junyu, et al. VOCemission inventory and its uncertainty from the key VOCrelated industries in the Pearl River Delta Region [J]. China Environmental Science, 2011, 31(02): 195-201.
[7] 李璇,王雪松,刘中,等.宁波人为源VOC清单及重点工业行业贡献分析[J].环境科学,2014, 35(07):2497-2502.
LI Xuan, WANG Xuesong, LIU Zhong, et al. Anthropogenic VOC emission inventory and contribution from industrial sources in Ningbo [J]. Environmental Science, 2014, 35(07): 2497-2502.
[8] 毛攀,吴秀才,赵瑜.南京市化工行业非甲烷挥发性有机物排放清单研究[J].中国科技论文,2015(12):1424-1430.
MAO Pan, WU Xiucai, ZHAO Yu. Study on emission inventory of nonmethane volatile organic compounds for chemical industry in Nanjing [J]. China Science Paper, 2015(12): 1424-1430.
[9] 黄玉虎,常耀卿,任碧琪,等.北京市19902030年加油站汽油VOCs排放清单[J].环境科学研究,2016,29(07): 945-951.
HUANG Yuhu, CHANG Yaoqing, REN Biqi, et al. Emissions inventory of gasoline VOCs from service stations in Beijing from 1990 to 2030 [J]. Research of Environmental Science, 2016, 29 (07): 945-951.
[10] 严茹莎,李莉,安静宇,等.夏季长三角地区臭氧非线性响应曲面模型的建立及应用[J].环境科学学报,2016, 36(04): 1383-1392.
YAN Rusha, LI li, AN Jingyu, et al. Establishment and application of nonlinear response surface model of ozone in the Yangtze River Delta region during summer time [J]. Acta Scientiae Circumstantiae, 2016, 36(04): 1383-1392.
[11] 杨杨,杨静,尹沙沙,等.珠江三角洲印刷行业VOCs组分排放清单及关键活性组分[J]. 环境科学研究, 2013, 26(03): 326-333.
YANG Yang, YANG Jing, YIN Shasha, et al. Speciated VOCs emission inventory and key species from printing industry in the Pearl River Delta region [J]. Research of Environmental Sciences, 2013, 26(03):326-333.
[12] 吴洪杰,刘玲英,蔡慧华,等.珠江三角洲制鞋行业挥发性有机化合物排放系数研究[J].中国环境监测, 2013(04): 74-78.
WU Hongjie, LIU Lingying, CAI Huihua, et al. Study on the emission coefficient of VOCs from shoemaking industry in the Pearl River Delta Region [J]. Environmental Monitoring in China, 2013(04):74-78.
[13] 王宇楠,叶代启,林俊敏,等.漆包线行业挥发性有机物(VOCs)排放特征研究[J].中国环境科学,2012,32(06): 980-987.
WANG Yunan, YE Daiqi, LIN Junmin, et al. A study on emission characteristics of volatile organic compounds (VOCs) from enameled wire industry [J]. China Environmental Science, 2012, 32(06):980-987.
[14] 何华飞,王浙明,许明珠,等.制药行业VOCs排放特征及控制对策研究:以浙江为例[J].中国环境科学,2012, 32(12): 2271-2277.
HE Huafei, WANG Zheming, XU mingzhu, et al. Studies on the emission characteristics and countermeasures of VOCs from pharmaceutical industry: based on Zhejiang Province [J]. China Environmental Science, 2012, 32(12): 2271-2277.
[15] 李勤勤,张志娟,李杨,等.石油炼化无组织VOCs的排放特征及臭氧生成潜力分析[J].中国环境科学,2016,36(05): 1323-1331.
LI Qinqin, ZHANG Zhijuan, LI Yang, et al. Characteristics and ozone formation potential of fugitive volatile organic compounds (VOCs) emitted from petrochemical industry in Pearl River Delta [J]. China Environmental Science, 2016, 36(05): 1323-1331.
[16] 蒲静娇.上海地区高污染条件下气象场及环境空气质量的数值模拟研究[D].上海:复旦大学,2007.
PU Jingjiao. Numerical simulation on meteorological charateristics and air quality in Shanghai area under highpolluted circumstances [D]. Shanghai: FudanUniversity, 2007.
[17] 国家统计局工业统计司.中国工业经济统计年鉴[M].北京:中国统计出版社.
[18] 国家统计局.中国统计年鉴[M].北京:中国统计出版社.
[19] 国研数据重点行业数据库[DB/OL].[2015-06-21].http:∥data.drcnet.com.cn/web/ChannelPage.aspx?chnId=4522&leafI=17345&channel=fzgypage&structureId=244&nodeId=17345&uid=99580745.
[20] 中国化学纤维工业协会行业运行统计数据[DB/OL]. [2015-04-01]. http:∥www.cfa.com.cn/tml tjsj/index.html.
[21] 中华人民共和国环境保护部.大气挥发性有机物源排放清单编制技术指南[EB/OL].[2014-08-19].
http:∥www.zhb.gov.cn/gkml/hbb/bgg/201408/W020140828351293705457.pdf.
[22] 何敏,王幸锐,韩丽.四川省大气固定污染源排放清单及特征[J]. 环境科学学报, 2013, 33(11): 3127-3137.
HE Min, WANG Xingrui, HAN Li. Air pollutionemission inventory and characteristics from stationary sources in Sichuan Province [J]. Acta Scientiae Circumstantiae, 2013, 33(11): 3127-3137.
[23] 夏思佳,赵秋月,李冰,等.江苏省人为源挥发性有机物排放清单[J].环境科学研究,2014, 27(02): 120-126.
XIA Sijia, ZHAO Qiuyue, LI Bing, et al. Anthropogenic source VOCs emission inventory of Jiangsu Province [J]. Research of Environmental Sciences, 2014, 27(02): 120126.
[24] 公私场所固定污染源申报空气污染防制费之挥发性有机物之行业制程排放系数、操作单元(含设备组件)排放系数、控制效率及其他计量规定[S].台湾:台湾环境保护署,2009.
[25] Chapter 6: Organic Chemical Process Industry, AP42, 5th Edition, Volume I/Clearing house for Emission Inventories and Emissions Factors/Technology Transfer Network/USEPA [EB/OL]. [20150418]. http:∥www.epa.gov/ttn/chief/ap42/ch06/final/c06s09.pdf.
[26] 杨利娴.我国工业源VOCs排放时空分布特征与控制策略研究[D].广州:华南理工大学,2012.
YANG Lixian. Study on temporalspatial characteristic and control strategy of industrial emissions of volatile organic compounds in China [D]. Guangzhou: South China University of Technology, 2012.

[1] 韦彦斐,周荣,周敏捷,高翔. 水泥炉窑SNCR-SCR联合脱硝中试实验研究[J]. 浙江大学学报(工学版), 2020, 54(10): 1986-1992.
[2] 王军明,赵兴亚,陈玲红,韩黎霞,高翔,岑可法. 氨对二次有机气溶胶光学特性的影响[J]. 浙江大学学报(工学版), 2020, 54(9): 1812-1818.
[3] 李康为,应方,陈玲红,郑仙珏,韩黎霞,吴学成,高翔,岑可法. 杭州市主城区VOCs污染特征及影响因素[J]. 浙江大学学报(工学版), 2019, 53(4): 671-683.
[4] 胡磊青,程军,王亚丽,刘建忠,周俊虎,岑可法. PVP改性PDMS/PAN中空纤维复合膜提升表面亲水性[J]. 浙江大学学报(工学版), 2019, 53(2): 228-233.
[5] 程军,刘建峰,张曦,张泽,田江磊,周俊虎,岑可法. 微藻水热提取油脂经脱氧断键制航油[J]. 浙江大学学报(工学版), 2019, 53(2): 214-219.
[6] 李清毅, 孟炜, 吴国潮, 张军, 朱松强, 胡达清, 郑成航, 高翔, 王汝能, 刘海蛟. 超低排放脱硝运行状态及稳定性评估[J]. 浙江大学学报(工学版), 2016, 50(12): 2303-2311.
[7] 朱燕群, 杨业, 黄建鹏, 林法伟, 马强, 徐超群, 王智化, 岑可法. 橡胶厂60000 m3/h炭黑干燥炉烟气臭氧脱硝试验研究[J]. 浙江大学学报(工学版), 2016, 50(10): 1865-1870.
[8] 张军, 李存杰, 郑成航, 翁卫国, 朱松强, 王丁振, 高翔, 岑可法. 筛板塔细颗粒物协同脱除特性实验[J]. 浙江大学学报(工学版), 2016, 50(8): 1516-1520.
[9] 邱珊, 陈聪, 邓凤霞, 冀雅婉, 丁晓, 马放. 石墨电极E Fenton法处理罗丹明B废水[J]. 浙江大学学报(工学版), 2016, 50(4): 704-713.
[10] 周斌,周昊,王建阳,岑可法. 神华煤灰掺混木屑灰在O2/CO2气氛下的烧结特性[J]. 浙江大学学报(工学版), 2016, 50(3): 468-476.
[11] 周旭萍, 方梦祥, 项群扬, 蔡丹云, 王涛, 骆仲泱. 氨基酸盐吸收二氧化碳过程的传质特性[J]. 浙江大学学报(工学版), 2016, 50(2): 312-319.
[12] 宋祖威, 仲兆平, 张波, 吕子婷, 丁宽. 玉米秸秆和聚丙烯共催化热解试验[J]. 浙江大学学报(工学版), 2016, 50(2): 333-340.
[13] 鲍强, 周昊, 刘建成, 朱国栋, 时伟, 岑可法.
新型CeO2-V2O5/TiO2-SiO2催化剂高效抗碱金属中毒性能
[J]. 浙江大学学报(工学版), 2015, 49(10): 1855-1862.
[14] 方梦祥, 江文敏, 王涛, 项群扬, 卢佳汇, 周旭萍. 基于实验的直接蒸气再生CO2系统模拟及优化[J]. 浙江大学学报(工学版), 2015, 49(8): 1565-1571.
[15] 陈艳萍,吴思明,卢慧剑,魏博伦,何奕,施耀. MW燃煤电厂钒钛系脱硝催化剂失活原因分析[J]. 浙江大学学报(工学版), 2015, 49(3): 564-570.